Simulation of atmospheric transport and droplet-thin film collisions in desorption electrospray ionization.

نویسندگان

  • Anthony B Costa
  • R Graham Cooks
چکیده

Computational fluid dynamics is used to model atmospheric transport and droplet-thin film (surface) collisions in desorption electrospray ionization; experimentally obtained droplet properties are replicated in the simulations while a "droplet pick-up" mechanism of analyte transport is confirmed.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Ion Transport and Focal Properties of an Ellipsoidal Electrode Operated at Atmospheric Pressure

Most frequently, ions are transported from ambient pressure and manipulated under low pressure conditions. While a vacuum environment is necessary to make precise measurements of an ion’s mass-to charge ratio, the ability to effectively control ion trajectories and spatially manipulate ions without the use of vacuum systems is of great interest in a number of different fields. Modifications to ...

متن کامل

Droplet Analysis with Electrospray Ionization Mass Spec- Trometry Using an Integrated Glass Microchip

ABSTRACT We describe an integrated microchip for droplet analysis with electrospray ionization mass spectrometry (ESI-MS). The chip integrated multiple modules of droplet generator, droplet extraction interface, and monolithic ESI-emitter. A novel droplet extraction interface based on a hydrophilic tongue structure was developed to transfer droplet from segmented phase to aqueous phase with hig...

متن کامل

Desorption Electrospray Ionization (DESI)

A new method of desorption ionization is described and applied to the ionization of various compounds, including peptides and proteins present on metal, polymer, and mineral surfaces. Desorption electrospray ionization (DESI) is carried out by directing electrosprayed charged droplets and ions of solvent onto the surface to be analyzed. The resulting mass spectra are similar to normal ESI mass ...

متن کامل

Nonresonant Femtosecond Laser Vaporization with Electrospray Postionization for <italic>ex vivo</italic> Plant Tissue Typing Using Compressive Linear Classification

T detection and identification of molecules within complex biological matrixes (i.e., plant tissue) requires homogenization, filtration, and liquid extraction of the sample to prepare for analysis using techniques such as gas chromatography/mass spectrometry (GC/MS), liquid chromatography-mass spectrometry (LC-MS), capillary electrophoresis-mass spectrometry (CE-MS), and LC-NMR. Direct analysis...

متن کامل

Evaluation of micro-electrospray ionization with ion mobility spectrometry/mass spectrometry

In recent years, the resolving power of ion mobility instruments has been increased significantly, enabling ion mobility spectrometry (IMS) to be utilized as an analytical separation technique for complex mixtures. In theory, decreasing the drift tube temperature results in increased resolution due to decreased ion diffusion. However, the heat requirements for complete ion desolvation with elec...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:
  • Chemical communications

دوره 38  شماره 

صفحات  -

تاریخ انتشار 2007